%0 Journal Article %T Lead isotopes as tracers of crude oil migration within deep crustal fluid systems %+ Laboratoire de Géologie de Lyon - Terre, Planètes, Environnement (LGL-TPE) %+ British Geological Survey [Edinburgh] %+ Laboratoire de Sciences de la Terre (LST) %+ British Geological Survey (BGS) %+ Geological Survey of Norway (NGU) %+ Norwegian Petroleum Directorate %+ IFP Energies nouvelles (IFPEN) %+ Geoscience Australia %A Fetter, Nadège %A Blichert-Toft, Janne %A Ludden, John %A Lepland, Aivo %A Sánchez Borque, Jorge %A Greenhalgh, Erica %A Garcia, Bruno %A Edwards, Dianne %A Telouk, Philippe %A Albarède, Francis %< avec comité de lecture %@ 0012-821X %J Earth and Planetary Science Letters %I Elsevier %V 525 %P 115747 %8 2019-11 %D 2019 %R 10.1016/j.epsl.2019.115747 %K Northern Europe %K oil migration %K Pb isotopes %K porous-media convection %K crude oil %K black shales %Z Environmental Sciences %Z Sciences of the Universe [physics]/Earth SciencesJournal articles %X Although Pb, U, and Th may be fractionated between crude oil and formation waters, Pb isotopes are not. This unique property makes Pb isotopes a particularly useful marker of hydrocarbon generation and migration. Here we show that Pb isotopes offer a new vision of long-range (secondary) oil migration relevant to the formation of oil fields. North Sea oils are largely generated from Jurassic black shales, yet their Pb isotopes are mixtures of Cenozoic to Proterozoic end-members. The same observation is made for crude oils from the Paris Basin, the Barents Sea, Libya, Kuwait, Kazakhstan, and Australia. Bulk Pb in crude oil therefore, for the most part, is foreign to its source rock(s). Our high-precision Pb isotope data on 195 crude oils worldwide, the first such data set in the published literature, and 17 Northern European black shales indicate that deep-seated Pb components originating beneath the source rocks are ubiquitous in crude oil. This implies that oil fields are embedded in basinal convective systems of hydrous fluids heated from below. Plumes of hot fluids rise from the lower thermal boundary layer, which Pb isotopes require douse the basement, into the core of the porous-flow convective cell where they dissolve the newly formed hydrocarbons sequestered in the source rocks. The fluids finally unload unmixed formation waters and crude oil at the base of the upper (conductive) boundary layer where they can be trapped in favorable sites. Based on these new insights we argue that Pb isotopes in crude oil constitute a good tracer of oil migration. %G English %2 https://ifp.hal.science/hal-02335910/document %2 https://ifp.hal.science/hal-02335910/file/1-s2.0-S0012821X1930439X-main.pdf %L hal-02335910 %U https://ifp.hal.science/hal-02335910 %~ UNIV-ST-ETIENNE %~ ENS-LYON %~ SDE %~ INSU %~ IFP %~ CNRS %~ UNIV-LYON1 %~ LGL-TPE %~ GIP-BE %~ UDL %~ UNIV-LYON